By configuration file, I meant MSQ file. The vemsv3.ini is what everyone has, it comes with MegaTune.
Judging by your datalog I'm surprised you haven't blown up the engine yet. I won't tell you how to tune, this is just my first reaction.
Your lambda target and actual lambda is very, very far away from each other. If you don't tune to make the actual reading match target, then your VE table will look very weird and the tuning won't make sense - they are both part of the fuel calculation.
I would advice you to make a complete upgrade to VemsTune and 1.1.x to get more control, but it might be confusing along the way (learn a new interface). A nice start would be to post your actual MSQ file and tell us which firmware version you're running.
If you're running an Audi S4 (an impression I got from another thread) then there are good known configuration files for the newer firmwares and VemsTune, and lots of other people here run these engines. Are you running a PnP ECU ?