With the data you have from the dyno runs and the logging you should be able to work out roughly the peak air consumption. With that and the pressure ratio, you should be able to roughly plot on the compressor map and see where it is in relation to the surge line. If it is close, the pressure spikes could be linked to rotating stall.
The thing with rotating stall is that it generates a pulsing discharge pressure but just about keeps pushing air. More worryingly induces loads on the compressor impeller that the shaft bearings were never designed for. The net result is failure. The other worrying thing is that rotating stall is less noticeable than a full on surge. If it surges you bloody well know it does.
I know somewhat about rotating stall and surge on centrifugal compressors with our machines at work, they are only about 100x the size of your turbocharger lol. Rotating stall and surge on these causes 10s of thousands of ££££s damage in a very short space of time
Good for us, bad for the customer
Just one other thing to consider is the compressor intake tract. If there is enough restriction here at max airflow the compressor eye can be subject to a vacuum, artificially increasing your pressure ratio, thus pushing it closer to surge. The discharge pressure is only one part of it, the suction pressure also needs to be considered, and why when talking about centrifugal compressors, pressure ratio is used.
PS. I hope you get it sorted. this sounds awesome especially with 600hp+ lol. Here's me with a poxy 1.3l pushing 200hp